纤维素基有机-无机纳米光催化复合材料制备及其水处理应用的研究进展

doi:10.13475/j.fzxb.20200607109

Abstract

Abstract:

With the aim of solving the agglomeration of traditional nano-sized photocatalysts particles that leads to low catalytic activity and recycling difficulty, it is imperative to promote the scalable application of advanced photocatalytic technology using cellulose based hybrid photocatalysts with high active site exposure, high dispersion and long-term stability. This review summarizes the recent progress in worldwide research on cellulose-based organic-inorganic photocatalysts nanohybrids. In terms of different cellulose forms, the fabrication and preparation principle of nanocellulose, cellulose-based membrane, cellulose-based aerogel and their application in the fields of water treatment are discussed. The prospect of cellulose based photocatalytic materials and the existing scientific questions and limitations are proposed. It is anticipated that this review can be used as a reference for preparation and industrialization of cellulose-based functional materials, especially in areas of environmental remediation.

Key words: cellulose-based functional material, environmental remediation, organic-inorganic nanohybrid, advanced oxidation technology, dyeing and printing wastewater treatment

CLC Number:

TS102.5

ZHANG Tingting, XU Kexin, JIN Mengtian, GE Shijie, GAO Guohong, CAI Yixiao, WANG Huaping. Recent progress in preparation of cellulose-based organic-inorganic photocatalysts nanohybrids and it's application in water treatment[J].Journal of Textile Research, 2021, 42(07): 175-183.

Figures/Tables 3

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References 57

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名称	制备方法	直径/nm	长度/nm	聚合度
CNF	机械法、 TEMPO氧化法	5~60	1 000~10 000	≥500
CNC	酸水解法	5~70	100~250	500~15 000
BC	细菌合成法	20~100	呈纤维网络结构	4 000~10 000

光催化材料	制备形态	污染物	光源(波长)	降解率/%	时间/min	参考文献
TiO₂/C/棉纤维素	纳米纤维	X-BR	紫外光	90.0	15	[31]
GO@TiO₂/纤维素	纳米纤维	IC MB	40 W紫外光 (320~400 nm)	99.8 98.3	150 250	[32]
C掺杂 ZnO/纤维素	纳米颗粒	MO	6 W (200~400 nm)	95.4	120	[33]
ZIF-8/CNC	纳米颗粒	MB	太阳光	99.8	300	[34]
ZnO/CuO/CNC	纳米颗粒	RB	20 W 紫外光	99.7	40	[35]
BiOBr/纤维素微晶	纳米颗粒	RhB	300 W氙灯(>420 nm)	90.0	70	[36]
g-C₃N₄/CA	膜	RhB	太阳光	99.0	150	[37]
TiO₂-Au/纤维素	膜	RhB	500 W氙灯(>400 nm)	94.99	300	[38]
H₄SiW₁₂O₄₀/CA	膜	MO	300 W 汞灯	94.6	120	[39]
TiO₂/PDA/BC	膜	MO RhB MB	500 W汞灯(>320 nm)	95.1 100.0 99.5	30 60 20	[40]
g-C₃N₄/纤维素	气凝胶	MB	350 W氙灯(>400 nm)	99.8	80	[41]
TiO₂/ CNF	气凝胶	MB	汞灯(365 nm)	98.1	20	[42]
Cu₂O/CBA	气凝胶	MB	350 W氙灯(>400 nm)	95.79	60	[43]
CuS/CBA	气凝胶	MB	500 W氙灯(>400 nm)	94.1	60	[44]
SiO₂-W_xTiO₂/纤维素	气凝胶	RhB	125 W汞灯(>400 nm)	95.0	120	[45]
β-FeOOH/纤维素	水凝胶	MB	300 W氙灯(>420 nm)	99.89	30	[46]

光催化材料	制备形态	污染物	光源	去除率/%	时间/min	参考文献
P25/CAM	一体式	Cr⁶⁺	1700 W氙弧灯(280~400 nm)	100	90	[49]
TiO₂/CNC	纳米颗粒	Cr⁶⁺	300 W氙弧灯(420 nm)	96	80	[50]
N掺杂C/纤维素	纳米颗粒	Cr⁶⁺	500 W氙灯(>420 nm)	80	300	[51]
ZnIn₂S₄/CNF	纳米颗粒	Cr⁶⁺	300 W氙灯(>420 nm)	100	90	[12]
BiOBr/CCNF	纳米颗粒	Cr⁶⁺	200 W LED灯	100	60	[52]
SWCNT/Fe₃O₄/TiO₂/壳聚糖/CA	纳米纤维	As⁵⁺和Cr⁶⁺	30 W UV灯(365 nm)	>95	60	[53]
g-C₃N₄/CA	薄膜	Cr⁶⁺	300 W氙灯(380~750 nm)	95	100	[37]

Recent progress in preparation of cellulose-based organic-inorganic photocatalysts nanohybrids and it's application in water treatment

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