生物炭在印染废水处理中的应用研究进展

doi:10.13475/j.fzxb.20240306802

Abstract

Abstract:

Significance Biochar materials were pyrolyzed from waste biomass with little or no oxygen. Due to their large specific surface area, controllable porous structure and stable chemical properties, biochar materials have attracted extensive attention from researchers in the field of agricultural soil remediation, greenhouse gas emission reduction, water pollution control and capacitor preparation. The application of biochars deriving from residual biomass in the printing and dyeing wastewater treatment can not only realize the resource utilization of waste biomass, but also decrease the costs of wastewater treatment. At the same time, the waste biomass utilization and the fixing effects for carbon elements can solve the problem of shortage of fossil resources, and help achieve the goal of “carbon neutrality”. The application of biochar in the treatment of printing and dyeing wastewater fit the idea of green development, which is one of the hot points of current research.

Progress To improve the application performances of biochar in printing and dyeing wastewater treatment, the recent research progress in biochars and their removal mechanism for typical pollutants were reviewed and summarized. The influences of activation-modification process for biochar on the treatment effects and regeneration capacity were discussed. Moreover, to the existing problems (such as the wide difference between biochars, poor pertinence of biochar for typical pollutants in printing and dyeing wastewater, and difficult regeneration of biochar after adsorption), the strategies such as establishing standard for biochar products, modifying biochar through functional group and pore structure, and developing composite biochar materials with adsorption-desorption ability were proposed in this paper.

Conclusion and Prospect The application of biochar prepared from waste biomass in the treatment of printing and dyeing wastewater, as a beneficial supplement to activated carbon, is beneficial for the environmental protection. However, some key problems still persist, such as the wide difference between biochars, poor pertinence of biochar for typical pollutants in printing and dyeing wastewater, and difficult regeneration of biochar after adsorption. How to regulate the adsorption properties of biochars and to achieve low-cost regeneration of biochar after adsorption are the key problems chanllenging large-scale application of biochar in wastewater treatment. From this review, it is hoped to improve the foundamental understanding for application and research of biochar materials in printing and dyeing wastewater treatment.

Key words: waste biomass, biochar, functional modification, printing and dyeing wastewater, wastewater treatment, adsorption-desorption

CLC Number:

TQ325

JIN Rushi, CHEN Wanming, LIU Guojin, LIU Chenghai, QI Dongming, ZHAI Shimin. Application progress in biochars in printing and dyeing wastewater treatment[J].Journal of Textile Research, 2025, 46(04): 235-243.

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References 57

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改性/活化方法	原料	热解温度/℃	比表面积/ (m²·g^-1)	最佳处理效果pH值	目标污染物	去除量/ (mg·g^-1)	去除机制	文献
蒸汽活化	蘑菇底物	800	322.0	6~10	结晶紫	1 057.0	孔隙填充,氢键、静电相互作用	[25]
KOH活化	软木	750	2 865.0	—	亚甲基蓝	1 103.7	孔隙填充,静电吸引、氢键和π-π相互作用	[26]
KOH活化	胶渣	700	860.5	—	Cr(Ⅵ)	—	—	[27]
HCl活化			85.9			—	—
ZnCl₂活化			694.0			325.5	静电相互作用,表面官能团络合,孔隙填充
H₃PO₄活化	棉纺废料	500	1 498.0	6~8	亚甲基蓝	240	孔隙填充,π-π相互作用,静电吸引	[28]
H₃PO₄活化	桉树废料	500	1 265.6	—	Cr(Ⅵ)	235.0	—	[29]
H₃PO₄活化+ 氮掺杂	桉树废料	500	1 654.4	2	Cr(Ⅵ)	260.0	孔隙填充、还原 Cr(Ⅵ)、静电吸引	[29]
K₂CO₃活化+ 氮参杂	废玉米芯	900	2 745.4	—	罗丹明B	1 630.7	氢键、静电吸引和 π-π相互作用	[30]
K₂CO₃活化+ 氮参杂	废玉米芯	900	2 745.4	—	刚果红	1 766.2	氢键、静电吸引和 π-π相互作用	[30]
NaOH活化+ 硫掺杂	平菇废料	500	47.6	7	Cd(Ⅱ)	56.0	离子交换,表面络合作用	[31]
磷掺杂	竹材	550	156.0	—	Cd(Ⅱ)	287.0	络合反应, 沉淀反应	[32]
TiO₂-Ag负载	竹片	500	51.7	—	亚甲基蓝	—	光催化降解	[33]
十二烷基苯磺酸改性+磁化	木屑粉末	550	506.3	6	罗丹明B	367.7	孔隙填充,静电吸引, 氢键,表面络合,疏水和π-π相互作用	[34]
月桂酸改性+ 磁化	花旗松	/	695.0	—	石油	3 000~11 000	疏水和π-π 相互作用	[35]
/	松针	800	—	—	1,4-二噁烷	—	过硫酸盐活化体系	[36]
铁/氮掺杂	麦秆	800	362.5	7	酸性橙	100	过硫酸盐活化体系
CeO₂负载	废纸,麦秆	500	59.0	2.5~6.5	活性红84	—	超声催化体系	[37]
铁掺杂	污泥	1 100	18.9	2~4	环丙沙星	—	类芬顿体系	[38]
TiO₂负载	巨藻	400	—	—	亚甲基蓝	74.3	光催化体系	[39]

生物炭原料	改性方法	再生方法	目标处理物	循环次数	再生效率/%	参考文献
造纸厂污水污泥	蒸汽活化	300 ℃热分解再生	亚甲基蓝	3	85	[48]
美人蕉	—	热分解再生	镉	—	—	[49]
凤尾草	Fe修饰	NaOH作为解吸剂	As(Ⅲ)	5	27	[50]
棉秆	—	HNO₃作为解吸剂	Pb(Ⅱ)	3	85	[51]
椰壳	Fe/N改性	HCl作为解吸剂	罗丹明B	—	—	[52]
香蕉皮	FeSO₄改性	乙醇作为解吸剂	亚甲基蓝	5	75~80	[53]
有机污泥	—	类芬顿体系	亚甲基蓝	4	88	[54]
废核桃壳	负载TiO₂	光催化体系	甲基橙	5	92	[55]

Application progress in biochars in printing and dyeing wastewater treatment

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